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Abstract Using Keck Planet Imager and Characterizer high-resolution (R∼ 35,000) spectroscopy from 2.29 to 2.49μm, we present uniform atmospheric retrievals for eight young substellar companions with masses of ∼10–30M_Jup, orbital separations spanning ∼50–360 au, andT_effbetween ∼1500 and 2600 K. We find that all companions have solar C/O ratios and metallicities to within the 1σ–2σlevel, with the measurements clustered around solar composition. Stars in the same stellar associations as our systems have near-solar abundances, so these results indicate that this population of companions is consistent with formation via direct gravitational collapse. Alternatively, core accretion outside the CO snowline would be compatible with our measurements, though the high mass ratios of most systems would require rapid core assembly and gas accretion in massive disks. On a population level, our findings can be contrasted with abundance measurements for directly imaged planets withm< 10M_Jup, which show tentative atmospheric metal enrichment compared to their host stars. In addition, the atmospheric compositions of our sample of companions are distinct from those of hot Jupiters, which most likely form via core accretion. For two companions withT_eff∼ 1700–2000 K (κAnd b and GSC 6214–210 b), our best-fit models prefer a nongray cloud model with >3σsignificance. The cloudy models yield 2σ−3σlowerT_efffor these companions, though the C/O and [C/H] still agree between cloudy and clear models at the 1σlevel. Finally, we constrain¹²CO/¹³CO for three companions with the highest signal-to-noise ratio data (GQ Lup b, HIP 79098b, and DH Tau b) and report $v\sin i$and radial velocities for all companions.